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  1. 学術雑誌論文

Synthesis of 2-Aryl-5-Nitropyridines by Three-Component Ring Transformation of 3,5-Dinitro-2-Pyridone

http://hdl.handle.net/10173/1477
http://hdl.handle.net/10173/1477
e3738fd9-e84f-4e7f-91ff-11b1badb7e0b
名前 / ファイル ライセンス アクション
28-12.pdf 28-12.pdf (422.6 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2017-03-24
タイトル
タイトル Synthesis of 2-Aryl-5-Nitropyridines by Three-Component Ring Transformation of 3,5-Dinitro-2-Pyridone
言語
言語 eng
キーワード
主題Scheme Other
主題 Biaryls
キーワード
主題Scheme Other
主題 Multicomponent reactions
キーワード
主題Scheme Other
主題 Nitrogen heterocycles
キーワード
主題Scheme Other
主題 Nitropyridines
キーワード
主題Scheme Other
主題 Ring transformation
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
著者 Le, Thi Song

× Le, Thi Song

Le, Thi Song

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Asahara, Haruyasu

× Asahara, Haruyasu

Asahara, Haruyasu

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Kobiro, Kazuya

× Kobiro, Kazuya

Kobiro, Kazuya

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Sugimoto, Ryuichi

× Sugimoto, Ryuichi

Sugimoto, Ryuichi

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Saigo, Kazuhiko

× Saigo, Kazuhiko

Saigo, Kazuhiko

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Nishiwaki, Nagatoshi

× Nishiwaki, Nagatoshi

Nishiwaki, Nagatoshi

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抄録
内容記述タイプ Abstract
内容記述 2-Arylated-5-nitropyridines were efficiently synthesized by a three-component ring transformation of 3,5-dinitro-2-pyridone with aromatic ketones in the presence of ammonium acetate, in which the dinitropyridone serves as a synthetic equivalent of an unstable nitromalonaldehyde. Although a 2,8-diazabicyclo[3.3.1]non-3-ene derivative was also formed as a byproduct, it was converted into nitropyridines under the reaction conditions, heating in the presence of ammonium acetate. This experimental fact implies that the former compound is a kinetically controlled product and the latter is a thermodynamically controlled product because of the aromatization. This method is applicable to various kinds of aryl and (hetero)aryl ketones to afford the corresponding (hetero)arylated pyridines in good to excellent yields.
書誌情報 Asian Journal of Organic Chemistry

巻 3, 号 3, p. 297-302, 発行日 2014-03
ISSN
収録物識別子タイプ ISSN
収録物識別子 2193-5807
DOI
関連タイプ isVersionOf
識別子タイプ DOI
関連識別子 10.1002/ajoc.201300282
権利
権利情報 This is the accepted version of the following article: Corrigendum: Synthesis of 2-Aryl-5-Nitropyridines by Three-Component Ring Transformation of 3,5-Dinitro-2-Pyridone Volume 4, Issue 2, 94, Article first published online: 2 February 2015, which has been published in final form at http://onlinelibrary.wiley.com/doi/10.1002/ajoc.201300282/abstract;jsessionid=660535A8C8D3756DDD98C38F7A495083.f04t03?systemMessage=Pay+per+view+article+purchase%28PPV%29+on+Wiley+Online+Library+will+be+unavailable+on+Saturday+11th+March+from+05%3A00-14%3A00+GMT+%2F+12%3A00-09%3A00+EST+%2F+13%3A00-22%3A00+SGT+for+essential+maintenance.++Apologies+for+the+inconvenience.. This article may be used for non-commercial purposes in accordance with the Wiley Self-Archiving Policy.
著者版フラグ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
出版者
出版者 John Wiley & Sons
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